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Kim, Richard Hahnkee ; Leem, Juyoung ; Muratore, Christopher ; Nam, SungWoo ; Rao, Rahul ; Jawaid, Ali ; Durstock, Michael ; McConney, Michael ; Drummy, Lawrence ; Rai, Rachel ; et al ( , Nanoscale)Low temperature synthesis of high quality two-dimensional (2D) materials directly on flexible substrates remains a fundamental limitation towards scalable realization of robust flexible electronics possessing the unique physical properties of atomically thin structures. Herein, we describe room temperature sputtering of uniform, stoichiometric amorphous MoS 2 and subsequent large area (>6.25 cm 2 ) photonic crystallization of 5 nm 2H-MoS 2 films in air to enable direct, scalable fabrication of ultrathin 2D photodetectors on stretchable polydimethylsiloxane (PDMS) substrates. The lateral photodetector devices demonstrate an average responsivity of 2.52 μW A −1 and a minimum response time of 120 ms under 515.6 nm illumination. Additionally, the surface wrinkled, or buckled, PDMS substrate with conformal MoS 2 retained the photoconductive behavior at tensile strains as high as 5.72% and over 1000 stretching cycles. The results indicate that the photonic crystallization method provides a significant advancement in incorporating high quality semiconducting 2D materials applied directly on polymer substrates for wearable and flexible electronic systems.more » « less
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Merrill, Nicholas A. ; Nitka, Tadeusz T. ; McKee, Erik M. ; Merino, Kyle C. ; Drummy, Lawrence F. ; Lee, Sungsik ; Reinhart, Benjamin ; Ren, Yang ; Munro, Catherine J. ; Pylypenko, Svitlana ; et al ( , ACS Applied Materials & Interfaces)